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acidulate (v.)

"make somewhat sour, flavor with an acid," 1704 (implied in acidulated), from Latin acidulus "slightly sour" (see acidulous) + -ate (2). Related: Acidulating; acidulent.

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Definitions of acidulate from WordNet

acidulate (v.)
make sour or more sour;
Synonyms: sour / acidify / acetify
From wordnet.princeton.edu