1963, "to reform a criminal," back-formation from decriminalization. Meaning "to make legal something that formerly had been illegal" was in use by 1970 (there are isolated instances back to 1867). Related: Decriminalized; decriminalizing.
decrepitation
decrepitude
decrescendo
decretory
decriminalization
decriminalize
decry
decrypt
decubitus
decuple
decussate