mid-14c., "relax;" late 14c., "to set free," from un- (2), used here emphatically, + loose (v.). Old English had unliesan "unloose, set free." Related: Unloosed; unloosing.
unloose your sneakers
unlisted
unlivable
unload
unlock
unlooked
unloose
unloved
unlovely
unlucky
unmade
unmake