c. 1600 (transitive), from un- (2) + ravel (v.). Intransitive from 1640s. "The prefix is either reversive or intensive, according as ravel is taken to mean 'tangle' or 'untangle'" [Century Dictionary]. Related: Unravelled; unravelling; unravellment.
unravel the thread
can you unravel the mystery?
the sweater unraveled
unquenchable
unquestionable
unquestioned
unquiet
unquote
unravel
unreachable
unread
unreadable
unready
unreal