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overpopulate (v.)

also over-populate, "to overrun with too many people," 1828 (implied in overpopulated), from over- + populate (v.). Related: Overpopulating. Overpopulous "over-populated" is attested from 1670s.

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Definitions of overpopulate from WordNet

overpopulate (v.)
cause to have too great a population;
Some towns in New Jersey are becoming overpopulated
From wordnet.princeton.edu